Modeling nonadiabatic enhancement of photosynthetic energy transfer using porphyrin dimers.
A commonality among many highly efficient light harvesting protein complexes is that they exhibit strong and persistent coherent spectral signatures that coincide with the early steps of the energy transport process. Due in part to the inherent …
Electronic-vibrational coupling is the driving force behind many fundamental photochemical processes, ranging from phonon-assisted carrier cooling in semiconductors to photoisomerization in proteins and molecular chromophores. Correlations between …